Interface-driven ferromagnetism within the quantum wells of a rare earth titanate superlattice

preprint2016arXivOpen access

Abstract

Here we present polarized neutron reflectometry measurements exploring thin film heterostructures comprised of a strongly correlated Mott state, GdTiO3_3, embedded with SrTiO3_3 quantum wells. Our results reveal that the net ferromagnetism inherent to the Mott GdTiO3_3 matrix propagates into the nominally nonmagnetic SrTiO3_3 quantum wells and tracks the magnetic order parameter of the host Mott insulating matrix. Beyond a well thickness of 5 SrO layers, the magnetic moment within the wells is dramatically suppressed, suggesting that quenched well magnetism comprises the likely origin of quantum critical magnetotransport in this thin film architecture. Our data demonstrate that the interplay between proximate exchange fields and polarity induced carrier densities can stabilize extended magnetic states within SrTiO3_3 quantum wells.

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