Abstract

Here, we present a temperature (TT) dependent comparison between field-effect and Hall mobilities in field-effect transistors based on few-layered WSe2_2 exfoliated onto SiO2_2. Without dielectric engineering and beyond a TT-dependent threshold gate-voltage, we observe maximum hole mobilities approaching 350 cm2^2/Vs at TT=300 K. The hole Hall mobility reaches a maximum value of 650 cm2^2/Vs as TT is lowered below ∼\sim 150 K, indicating that insofar WSe2_2-based field-effect transistors (FETs) display the largest Hall mobilities among the transition metal dichalcogenides. The gate capacitance, as extracted from the Hall-effect, reveals the presence of spurious charges in the channel, while the two-terminal sheet resistivity displays two-dimensional variable-range hopping behavior, indicating carrier localization induced by disorder at the interface between WSe2_2 and SiO2_2. We argue that improvements in the fabrication protocols as, for example, the use of a substrate free of dangling bonds are likely to produce WSe2_2-based FETs displaying higher room temperature mobilities, i.e. approaching those of pp-doped Si, which would make it a suitable candidate for high performance opto-electronics.

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