Ghost modes and continuum scattering in the dimerized distorted kagome lattice antiferromagnet Rb2_2Cu3_3SnF12_{12}

preprint2013arXivOpen access

Abstract

High intensity pulsed neutron scattering reveals a new set of magnetic excitations in the pinwheel valence bond solid state of the distorted kagome lattice antiferromagnet Rb2_2Cu3_3SnF12_{12}. The polarization of the dominant dispersive modes (2 meV <ℏω<<\hbarω< 7 meV) is determined and found consistent with a dimer series expansion with strong Dzyaloshinskii-Moriya interactions (D/J=0.18D/J=0.18). A weakly dispersive mode near 5 meV and shifted "ghosts" of the main modes are attributed to the enlarged unit cell below a T=215T=215 K structural transition. Continuum scattering between 8 meV and 10 meV might be interpreted as a remnant of the kagome spinon continuum [T.-H. Han et al., Nature 492, 406 (2012)]

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