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Electronic structure of CaFe2As2: Contribution of itinerant Fe 3d-states to the Fermi Level

We present density functional theory (DFT) calculations and a full set of X-ray spectra (resonant inelastic X-ray scattering and X-ray photoelectron spectra) measurements of single crystal CaFe2As2. The experimental valence band spectra are consistent with our DFT calculations. Both theory and experiment show that the Fe 3d-states dominate the Fermi level and hybridize with Ca 3d-states. The simple shape of Xray photoelectron (XPS) Fe 2p-core level spectrum (without any satellite structure typical for correlated systems) suggests itinerant character of the Fe 3d-electrons. Based on the similarity of the calculated and experimental Fe 3d-states distribution in LaOFeAs and CaFe2As2 we conclude that superconductivity in the FeAs-systems can be described within a minimal model, taking into account only Fe 3d-bands close to the Fermi level.

preprint2009arXivOpen access
E. Z. KurmaevJ. A. McLeodA. BulingN. A. SkorikovA. MoewesM. NeumannM. A. KorotinYu. A. IzyumovN. NiP. C. Canfield
cond-mat.supr-con
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E. Z. KurmaevJ. A. McLeodA. BulingN. A. SkorikovA. MoewesM. NeumannM. A. KorotinYu. A. IzyumovN. NiP. C. Canfield

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