Decoupling and tuning competing effects of different types of defects on flux creep in irradiated YBa2_{2}Cu3_{3}O7−δ_{7-δ} coated conductors

preprint2016arXivOpen access

Abstract

YBa2_{2}Cu3_{3}O7−δ_{7-δ} coated conductors (CCs) have achieved high critical current densities (Jc\textit{J}_{c}) that can be further increased through the introduction of additional defects using particle irradiation. However, these gains are accompanied by increases in the flux creep rate, a manifestation of competition between the different types of defects. Here, we study this competition to better understand how to design pinning landscapes that simultaneously increase Jc\textit{J}_{c} and reduce creep. CCs grown by metal organic deposition show non-monotonic changes in the temperature-dependent creep rate, S(T)\textit{S}(\textit{T}). Notably, in low fields, there is a conspicuous dip to low S\textit{S} as temperature (T\textit{T}) increases from ~20 K to ~65 K. Oxygen-, proton-, and Au-irradiation substantially increase S\textit{S} in this temperature range. Focusing on an oxygen-irradiated CC, we investigate the contribution of different types of irradiation-induced defects to the flux creep rate. Specifically, we study S(T)\textit{S}(\textit{T}) as we tune the relative density of point defects to larger defects by annealing both an as-grown and an irradiated CC in O2_{2} at temperatures TA\textit{T}_{A} = 250°°C to 600°°C. We observe a steady decrease in S\textit{S}(T\textit{T} > 20 K) with increasing TA\textit{T}_{A}, unveiling the role of pre-existing nanoparticle precipitates in creating the dip in S(T)\textit{S}(\textit{T}) and point defects and clusters in increasing S\textit{S} at intermediate temperatures.

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