Abstract

Decay spectroscopy of the long-lived states in 186^{186}Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The αα decay from the low-spin (2−)(2^-) state in 186^{186}Tl was observed for the first time and a half-life of 3.4−0.4+0.53.4^{+0.5}_{-0.4} s was determined. Based on the αα-decay energy, the relative positions of the long-lived states were fixed, with the (2−)(2^-) state as the ground state, the 7(+)7^{(+)} state at 77(56)~keV and the 10(−)10^{(-)} state at 451(56) keV. The level scheme of the internal decay of the 186^{186}Tl(10(−)10^{(-)}) state (T1/2=3.40(9)T_{1/2} = 3.40(9) s), which was known to decay solely through emission of 374 keV γγ-ray transition, was extended and a lower-limit for the ββ-decay branching bβ>5.9(3)%b_β> 5.9(3)\% was determined. The extracted retardation factors for the γγ decay of the 10(−)10^{(-)} state were compared to the available data in neighboring odd-odd thallium isotopes indicating the importance of the πd3/2πd_{3/2} shell in the isomeric decay and significant structure differences between 184^{184}Tl and 186^{186}Tl.

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