Critical temperature and low-energy excitations in gapped spin systems with defects

preprint2021arXivOpen access

Abstract

We discuss theoretically the magnetically ordered phase induced by magnetic and nonmagnetic impurities in three-dimensional and quasi-low-dimensional systems with singlet ground states separated by a gap from excited triplet states. Using ideas of the percolation theory, we estimate the transition temperature TN(n)T_N(n) to the Néel phase at a small concentration nn of defects, derive the density of states of low-energy elementary excitations, and examine the contribution of these excitations to the specific heat and magnetization. Our expressions for TN(n)T_N(n) and for the specific heat describe well available experimental findings obtained in various appropriate systems: spin-12\frac12 dimer materials, spin-ladder compounds, spin-Peierls and Haldane chain materials. However, our expression for TN(n)T_N(n) differs considerably from many of those proposed before.

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