Counter-rotating spiral, zigzag, and 120∘^\circ orders from coupled-chain analysis of Kitaev-Gamma-Heisenberg model, and relations to honeycomb iridates

preprint2022arXivOpen access

Abstract

We study the nearest neighboring spin-1/2 Kitaev-Heisenberg-Gamma (KJΓKJΓ) model on the honeycomb lattice in the parameter region of ferromagnetic (FM) Kitaev and antiferromagnetic (AFM) Heisenberg couplings relevant for honeycomb iridates, using a coupled-chain analysis. Starting from the gapless Luttinger liquid phase of a decoupled KJΓKJΓ chain, the inter-chain interactions in the two-dimensional model is treated within a self-consistent mean field approach based on the Luttinger liquid theory. In the FM Gamma region, our analysis recovers the reported 120∘^\circ magnetic order, previously obtained by classical analysis and exact diagonalization method. On the other hand, new physics is revealed in the AFM Gamma region, where three magnetic orders are found, including 120∘^\circ, commensurate counter-rotating spiral, and zigzag orders. Interestingly, the two first order phase transition lines separating these three magnetic orders merge at a single point at K=−2ΓK = -2 Γ and J=0J=0, which is predicted to be a quantum critical point. The current theory captures the experimentally observed counter-rotating spiral order in αα-Li22_22IrO3_3 and the zigzag order in Na2_2IrO3_3, thereby indicating that the spin-1/2 KJΓKJΓ model may serve as a minimal model for honeycomb iridates. Limitations of the mean field theory presented in this work and the J→0J \rightarrow 0 regime are also discussed.

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