Complex magnetic order in YbMn2_2Sb2_2 single crystals observed by μμSR

preprint2020arXivOpen access

Abstract

The crystal growth and the structural, transport and magnetic properties of the magnetically frustrated YbMn2_2Sb2_2 single crystals are reported. The crystals show a trigonal symmetry (space group P3ˉm1P\bar{3}m1), where corrugated honeycomb layers of MnSb are separated by Yb atoms. No structural phase transition was observed down to 22~K. The resistivity measurements show a predominantly insulating behavior. The combined resistivity, dc susceptibility and heat capacity measurements confirm successive transitions at 230~K, 116~K and 27~K, being the transition at TNT_N=116~K due to the Mn+2^{+2} lattice antiferromagnetic ordering. Muon spin rotation experiments (μμSR) reveal a more complicated scenario, with temperature dependence of the magnetic volume fraction reflecting short range and long range magnetic order, and a strongly disordered magnetic ground state. The role of spin-lattice coupling and its relationship with exchange interactions between Mn moments are discussed as possible cause of the complex magnetic behavior observed.

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