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Complex magnetic order in YbMn$_2$Sb$_2$ single crystals observed by $μ$SR

The crystal growth and the structural, transport and magnetic properties of the magnetically frustrated YbMn$_2$Sb$_2$ single crystals are reported. The crystals show a trigonal symmetry (space group $P\bar{3}m1$), where corrugated honeycomb layers of MnSb are separated by Yb atoms. No structural phase transition was observed down to 22~K. The resistivity measurements show a predominantly insulating behavior. The combined resistivity, dc susceptibility and heat capacity measurements confirm successive transitions at 230~K, 116~K and 27~K, being the transition at $T_N$=116~K due to the Mn$^{+2}$ lattice antiferromagnetic ordering. Muon spin rotation experiments ($μ$SR) reveal a more complicated scenario, with temperature dependence of the magnetic volume fraction reflecting short range and long range magnetic order, and a strongly disordered magnetic ground state. The role of spin-lattice coupling and its relationship with exchange interactions between Mn moments are discussed as possible cause of the complex magnetic behavior observed.

preprint2020arXivOpen access
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