Coexisting pseudogap, charge transfer gap, and Mott gap energy scales in the resonant inelastic x-ray scattering spectra of electron-doped cuprates

preprint2012arXivOpen access

Abstract

We present a computation of Cu K-edge resonant inelastic x-ray scattering (RIXS) spectra for electron-doped cuprates which includes coupling to bosonic fluctuations. Comparison with experiment over a wide range of energy and momentum transfers allows us to identify the signatures of three key normal-state energy scales: the pseudogap, charge transfer gap, and Mott gap. The calculations involve a three band Hubbard Hamiltonian based on Cu dx2−y2d_{x^2-y^2} and O pxp_x, pyp_y orbitals, with a self-energy correction which arises due to spin and charge fluctuations. Our theory reproduces characteristic features e.g., gap collapse, large spectral weight broadening, and spectral weight transfer as a function of doping, as seen in experiments.

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