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Paper detail

Broadband high-resolution two-photon spectroscopy with laser frequency combs

Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb technique. Each transition is uniquely identified by the modulation imparted by the interfering comb excitations. The temporal modulation of the spontaneous two-photon fluorescence is monitored with a single photodetector, and the spectrum is revealed by a Fourier transform.

preprint2013arXivOpen access
Arthur HipkeSamuel A. MeekTakuro IdeguchiTheodor W. HänschNathalie Picqué
physics.optics
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Arthur HipkeSamuel A. MeekTakuro IdeguchiTheodor W. HänschNathalie Picqué

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