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Avoiding Stripe Order: Emergence of the Supercooled Electron Liquid

In the absence of disorder, electrons can display glassy behavior through supercooling the liquid state, avoiding the solidification into a charge ordered state. Such supercooled electron liquids are experimentally found in organic $θ$-$MM'$ compounds. We present theoretical results that qualitatively capture the experimental findings. At intermediate temperatures, the conducting state crosses over into a weakly insulating pseudogap phase. The stripe order phase transition is first order, so that the liquid phase is metastable below $T_s$. In the supercooled liquid phase the resistivity increases further and the density of states at the Fermi level is suppressed, indicating kinetic arrest and the formation of a glassy state. Our results are obtained using classical Extended Dynamical Mean Field Theory.

preprint2016arXivOpen access
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