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ARPES in strongly disordered systems -- theory of electronic bands melting

It is well known that translational symmetry-breaking disorder will disrupt ARPES spectra up to the point where they become invisible. However, a theoretical framework to capture this phenomenon has been largely missing. Here, based on a rigorous theory of the ARPES process, we provide this much-needed framework. In particular, we show how the frequently used sudden electron approximation has to be modified in this situation. Our main result is an argument that links the photoemission line broadening with an operator content of a disorder operator and so with the criticality of the corresponding order-disorder phase transition. For concreteness, we focus here on the frustrated 2D trigonal (pseudo-)spin model, with Ising order-disorder operators behind the transition. Still, our formalism is general and can be applied in a much broader context.

preprint2022arXivOpen access

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