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Anomalous Hall effect at the spontaneously electron-doped polar surface of PdCoO2 ultrathin films

We revealed the electrical transport through surface ferromagnetic states of a nonmagnetic metal PdCoO2. Electronic reconstruction at the Pd-terminated surface of PdCoO2 induces Stoner-like ferromagnetic states, which could lead to spin-related phenomena among the highly conducting electrons in PdCoO2. Fabricating a series of nanometer-thick PdCoO2 thin films, we detected a surface-magnetization-driven anomalous Hall effect via systematic thickness- and termination-dependent measurements. Besides, we discuss that finite magnetic moments in electron doped CoO2 triangular lattices may have given rise to additional unconventional Hall resistance.

preprint2019arXivOpen access
T. HaradaK. SugawaraK. FujiwaraS. ItoT. NojimaT. TakahashiT. SatoA. Tsukazaki
cond-mat.str-elcond-mat.mtrl-sci
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Open access8 authors2 topics
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T. HaradaK. SugawaraK. FujiwaraS. ItoT. NojimaT. TakahashiT. SatoA. Tsukazaki

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