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Angle-resolved photoemission spectroscopy with 9-eV photon-energy pulses generated in a gas-filled hollow-core photonic crystal fiber

A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet (VUV) radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi2Se3 with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz, with photon energies that cover the first Brillouin zone of most materials.

preprint2015arXivOpen access
H. BrombergerA. ErmolovF. BelliH. LiuF. CalegariM. Chavez-CervantesM. T. LiC. T. LinA. AbdolvandP. St. J. RussellA. CavalleriJ. C. TraversI. Gierz
physics.optics
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Open access13 authors1 topic
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H. BrombergerA. ErmolovF. BelliH. LiuF. CalegariM. Chavez-CervantesM. T. LiC. T. LinA. AbdolvandP. St. J. RussellA. CavalleriJ. C. TraversI. Gierz

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