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13C NMR study of the magnetic properties of the quasi-one-dimensional conductor, (TMTTF)2SbF6

Magnetic properties in the quasi-one-dimensional organic salt (TMTTF)2SbF6 are investigated by 13C NMR under pressures. Antiferromagnetic phase transition at ambient pressure (AFI) is confirmed. Charge-ordering is suppressed by pressure and is not observed under 8 kbar. For 5 < P < 20 kbar, a sharp spectrum and the rapid decrease of the spin-lattice relaxation rate 1/T1 were observed below about 4 K, attributed to a spin-gap transition. Above 20 kbar, extremely broadened spectrum and critical increase of 1/T1 were observed. This indicates that the system enters into another antiferromagnetic phase (AFII) under pressure. The slope of the antiferromagnetic phase transition temperature T_AFII, dT_AFII/dP, is positive, while T_AFI decreases with pressure. The magnetic moment is weakly incommensurate with the lattice at 30 kbar.

preprint2011arXivOpen access
F. IwaseK. SugiuraK. FurukawaT. Nakamura
cond-mat.str-el
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F. IwaseK. SugiuraK. FurukawaT. Nakamura

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