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Unconventional Magnetism in a Nitrogen-Based Analogue of Cupric Oxide

We have investigated the magnetic properties of CuNCN, the first nitrogen-based analogue of cupric oxide, CuO. Our muon spin relaxation, nuclear magnetic resonance and electron spin resonance studies reveal that classical magnetic ordering is absent down to lowest temperatures. However, large enhancement of spin correlations and unexpected inhomogeneous magnetism have been observed below 80 K. We attribute this to a peculiar fragility of the electronic state against weak perturbations due to geometrical frustration, which selects between competing spin-liquid and more conventional frozen states.

preprint2011arXivOpen access
A. ZorkoP. JegličA. PotočnikD. ArčonA. BalčytisZ. JagličićX. LiuA. L. TchougréeffR. Dronskowski
cond-mat.str-el
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Open access9 authors1 topic
Imported metadata coverageMissing code, dataset, citation and institution fields are tracked without dominating the paper.Details
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A. ZorkoP. JegličA. PotočnikD. ArčonA. BalčytisZ. JagličićX. LiuA. L. TchougréeffR. Dronskowski

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