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Paper detail

Two-body tunnel transitions in a Mn4 Single-Molecule Magnet

The one-body tunnel picture of single-molecule magnets (SMMs) is not always sufficient to explain the measured tunnel transitions. An improvement to the picture is proposed by including also two-body tunnel transitions such as spin-spin cross-relaxation (SSCR) which are mediated by dipolar and weak superexchange interactions between molecules. A Mn4 SMM is used as a model system. At certain external fields, SSCRs lead to additional quantum resonances which show up in hysteresis loop measurements as well defined steps.

preprint2003arXivOpen access
W. WernsdorferS. BhaduriR. TironD. N. HendricksonG. Christou
cond-mat.stat-mechcond-mat.mes-hall
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W. WernsdorferS. BhaduriR. TironD. N. HendricksonG. Christou

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