Thermodynamic properties of an S=1/2S=1/2 ring-exchange model on the triangular lattice

preprint2020arXivOpen access

Abstract

By using a numerically exact diagonalization technique and a block-extended version of the finite-temperature Lanczos method, we study thermodynamic properties of an S=1/2S=1/2 Heisenberg model on the triangular lattice with an antiferromagnetic nearest-neighbor interaction JJ and a four-spin ring-exchange interaction JcJ_{\rm c}. Calculations are performed on small clusters under the periodic-boundary conditions. In contrast to the purely triangular case with Jc=0J_{\rm c}=0, the specific heat exhibits a characteristic double-peak structure for Jc/J≳0.04J_{\rm c}/J \gtrsim 0.04. From the calculation of the entropy and the uniform magnetic susceptibility, it is shown that non-magnetic excitations exist below the magnetic excitation for Jc/J≳0.04J_{\rm c}/J \gtrsim 0.04.

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