The chain sucker: translocation dynamics of a polymer chain into a long narrow channel driven by longitudinal flow

preprint2011arXivOpen access

Abstract

Using analytical techniques and Langevin dynamics simulations, we investigate the dynamics of polymer translocation into a narrow channel of width RR embedded in two dimensions, driven by a force proportional to the number of monomers in the channel. Such a setup mimics typical experimental situations in nano/micro-fluidics. During the the translocation process if the monomers in the channel can sufficiently quickly assume steady state motion, we observe the scaling τ∼N/Fτ\sim N/F of the translocation time ττ with the driving force FF per bead and the number NN of monomers per chain. With smaller channel width RR, steady state motion cannot be achieved, effecting a non-universal dependence of ττ on NN and FF. From the simulations we also deduce the waiting time distributions under various conditions for the single segment passage through the channel entrance. For different chain lengths but the same driving force, the curves of the waiting time as a function of the translocation coordinate ss feature a maximum located at identical smaxs_{\mathrm{max}}, while with increasing the driving force or the channel width the value of smaxs_{\mathrm{max}} decreases.

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