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Terahertz response of gadolinium gallium garnet (GGG) and gadolinium scandium gallium garnet (SGGG)

We report the magneto-optical response of Gadolinium Gallium Garnet (GGG) and Gadolinium Scandium Gallium Garnet (SGGG) at frequencies ranging from $300 \, \mathrm{GHz}$ to $1 \, \mathrm{THz}$, and determine the material response tensor. Within this frequency window, the materials exhibit nondispersive and low-loss optical responses. At low temperatures, significant THz Faraday rotations are found in the (S)GGG samples. Such strong gyroelectric response is likely associated with the high-spin paramagnetic state of the Gd$^{3+}$ ions. A model of the material response tensor is determined, together with the Verdet and magneto-optic constants.