Symmetric and antisymmetric exchange anisotropies in quasi-one-dimensional CuSe2_2O5_5 as revealed by ESR

preprint2011arXivOpen access

Abstract

We present an electron spin resonance (ESR) study of single-crystalline spin chain-system CuSe2_2O5_5 in the frequency range between 9 GHz and 450 GHz. In a wide temperature range above the Néel temperature TN=17T_N=17 K we observe strong and anisotropic frequency dependence of a resonance linewidth. Although sizeable interchain interaction JIC≈0.1JJ_{IC}\approx 0.1 J (JJ is the intrachain interaction) is present in this system, the ESR results agree well with the Oshikawa-Affleck theory for one-dimensional S=1/2S=1/2 Heisenberg antiferromagnet. This theory is used to extract the anisotropies present in CuSe2_2O5_5. We find that the symmetric anisotropic exchange Jc=(0.04±0.01) JJ_c=(0.04 \pm 0.01) \:J and the antisymmetric Dzyaloshinskii-Moriya (DM) interaction D=(0.05±0.01) JD=(0.05\pm 0.01)\:J are very similar in size in this system. Staggered-field susceptibility induced by the presence of the DM interaction is witnessed in the macroscopic susceptibility anisotropy.

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