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Spontaneous emission enhancement of a single molecule by a double-sphere nanoantenna across an interface

We report on two orders of magnitude reduction in the fluorescence lifetime when a single molecule placed in a thin film is surrounded by two gold nanospheres across the film interface. By attaching one of the gold particles to the end of a glass fiber tip, we could control the modification of the molecular fluorescence at will. We find a good agreement between our experimental data and the outcome of numerical calculations.

preprint2012arXivOpen access
K. -G. LeeH. EghlidiX-W. ChenA. RennS. GötzingerV. Sandoghdar
physics.opticsquant-ph
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Open access6 authors2 topics
Imported metadata coverageMissing code, dataset, citation and institution fields are tracked without dominating the paper.Details
Citations: 0Reviews: 0Saves: 0Code: not linkedDataset: not linkedInstitutions: 0

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K. -G. LeeH. EghlidiX-W. ChenA. RennS. GötzingerV. Sandoghdar

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