Spin Wave Analysis of Low-Temperature Thermal Hall Effect in the Candidate Kitaev Spin Liquid αα-RuCl3{}_3

preprint2018arXivOpen access

Abstract

Proposed effective Hamiltonians from the literature for the material αα-RuCl3{}_3 are used to compute the magnon thermal Hall conductivity, κxyκ_{xy}, using linear spin wave theory for the magnetically ordered state. No model previously proposed that was tested explains published experimental data. Models with Kitaev interaction K>0K>0 are seen to predict κxy≳0κ_{xy}\gtrsim 0, which is inconsistent with the data. Fluctuations toward a Kitaev-type spin liquid would have the wrong sign to explain the data. However, a slight variant of a previously proposed model predicts a large κxyκ_{xy}, demonstrating that the low-temperature thermal Hall effect could be generated exclusively by the Berry curvature of the magnon bands. The experimental data of κxyκ_{xy} can therefore serve as another method to constrain a proposed effective Hamiltonian.

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