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Spin Wave Analysis of Low-Temperature Thermal Hall Effect in the Candidate Kitaev Spin Liquid $α$-RuCl${}_3$

Proposed effective Hamiltonians from the literature for the material $α$-RuCl${}_3$ are used to compute the magnon thermal Hall conductivity, $κ_{xy}$, using linear spin wave theory for the magnetically ordered state. No model previously proposed that was tested explains published experimental data. Models with Kitaev interaction $K>0$ are seen to predict $κ_{xy}\gtrsim 0$, which is inconsistent with the data. Fluctuations toward a Kitaev-type spin liquid would have the wrong sign to explain the data. However, a slight variant of a previously proposed model predicts a large $κ_{xy}$, demonstrating that the low-temperature thermal Hall effect could be generated exclusively by the Berry curvature of the magnon bands. The experimental data of $κ_{xy}$ can therefore serve as another method to constrain a proposed effective Hamiltonian.

preprint2018arXivOpen access
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