{Spin polarization tuning in Mnx_{x}Fe1−x_{1-x}Ge3_{3}

preprint2008arXivOpen access

Abstract

Experimentally, the intermetallic compound Mn4_{4}FeGe3_{3} has been recently shown to exhibit enhanced magnetic properties and spin polarization compared to the Mn5_{5}Ge3_{3} parent compound. The present {\em ab-initio} study focusses on the effect of Fe substitution on the electronic and magnetic properties of the compound. Our calculations reveal that the changes on the Fermi surface of the doped compound are remarkable and provide explanations for the enhanced spin-polarization observed. Finally, we show that it is indeed possible to tune the degree of spin-polarization upon Fe doping, thus making the Mn1−x_{1-x}Fex_{x}Ge3_{3} intermetallic alloy very promising for future spintronic applications.

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