Spin-pairing and penetration depth measurements from nuclear magnetic resonance in NaFe0.975_{0.975}Co0.025_{0.025}As

preprint2013arXivOpen access

Abstract

We have performed 75^{75}As nuclear magnetic resonance (NMR) Knight shift measurements on single crystals of NaFe0.975_{0.975}Co0.025_{0.025}As to show that its superconductivity is a spin-paired, singlet state consistent with predictions of the weak-coupling BCS theory. We use a spectator nucleus, 23^{23}Na, uncoupled from the superconducting condensate, to determine the diamagnetic magnetization and to correct for its effect on the 75^{75}As NMR spectra. The resulting temperature dependence of the spin susceptibility follows the Yosida function as predicted by BCS for an isotropic, single-valued energy gap. Additionally, we have analyzed the 23^{23}Na spectra that become significantly broadened by vortices to obtain the superconducting penetration depth as a function of temperature with λab(0)=5,327±λ_{ab}(0) = 5,327 \pm 78 A˚\,Å.

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