Spatial behavior in a Mott insulator near the voltage-driven resistive transition

preprint2020arXivOpen access

Abstract

We develop a real space theory of the voltage bias driven transition from a Mott insulator to a correlated metal. Within our Keldysh mean field approach the problem reduces to a self-consistency scheme for the charge and spin profiles in this open system. We solve this problem for a two dimensional antiferromagnetic Mott insulator at zero temperature. The charge and spin magnitude is uniform over the system at zero bias, but a bias VV leads to spatial modulation over a lengthscale ξ(V)ξ(V) near the edges. ξ(V)ξ(V) grows rapidly and becomes comparable to system size as VV increases towards a threshold scale VcV_c. The linear response conductance of the insulator is zero with the current being exponentially small for V≪VcV \ll V_c. The current increases rapidly as V→VcV \rightarrow V_c. Beyond VcV_c, we observe an inhomogeneous low moment antiferromagnetic metal, and at even larger bias a current saturated paramagnetic metal. We suggest an approximate scheme for the spectral features of this nonequilibrium system.

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