Site-dependent Local Spin Susceptibility and Low-energy Excitation in a Weyl Semimetal WTe2_2

preprint2022arXivOpen access

Abstract

Site-dependent local spin susceptibility is investigated with 125^{125}Te nuclear magnetic resonance in a Weyl semimetal WTe2_2. The nuclear spin-lattice relaxation rate 1/T1T1/T_1T shows a dependence of the square of temperature TT at high temperatures, followed by a constant behavior below 50 K. The temperature dependence features Weyl fermions appearing around the linearly crossing bands. The Knight shift KK scales to the square root of 1/T1T1/T_1T, corroborating a predominant spin contribution in low-lying excitation. The observed dependence of KK and 1/T1T1/T_1T on the four Te sites shows the site-dependent electron correlation and density of states. The angular profile of the NMR spectrum gives the anisotropic hyperfine coupling tensor, consistent with 5p5p hole occupations on Te sites.

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