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Single Crystal Study of Competing Rhombohedral and Monoclinic Order in Lead Zirconate Titanate

Neutron diffraction data obtained on single crystals of PbZr1-xTixO3 with x = 0.325 and x = 0.460, which lie on the pseudorhombohedral side of the morphotropic phase boundary, suggest a coexistence of rhombohedral (R3m/R3c) and monoclinic (Cm) domains and that monoclinic order is enhanced by Ti substitution. A monoclinic phase with a doubled unit cell (Cc) is ruled out as the ground state.

preprint2010arXivOpen access
D. PhelanX. LongY. XieZ. -G. YeA. M. GlazerH. YokotaP. A. ThomasP. M. Gehring
cond-mat.mtrl-sci
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D. PhelanX. LongY. XieZ. -G. YeA. M. GlazerH. YokotaP. A. ThomasP. M. Gehring

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