Abstract

We present experimental results for the heavy-electron compound CeCu4_{4}Ga which show that it possesses short-range magnetic correlations down to a temperature of T=0.1T = 0.1 K. Our neutron scattering data show no evidence of long-range magnetic order occurring despite a peak in the specific heat at T∗=1.2T^{*} =1.2 K. Rather, magnetic diffuse scattering occurs which corresponds to short-range magnetic correlations occurring across two unit cells. The specific heat remains large as T∼0T\sim0 K resulting in a Sommerfeld coefficient of γ0=1.44(2)γ_{0} = 1.44(2) J/mol-K2^{2}, and, below T∗T^{*}, the resistivity follows T2T^{2} behavior and the ac magnetic susceptibility becomes temperature independent. A magnetic peak centered at an energy transfer of Ec=0.24(1)E_{\rm{c}}=0.24(1) meV is seen in inelastic neutron scattering data which shifts to higher energies and broadens under a magnetic field. We discuss the coexistence of large specific heat, magnetic fluctuations, and short-range magnetic correlations at low temperatures and compare our results to those for materials possessing spin-liquid behavior.

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