Role of commensurate and incommensurate low-energy excitations in the paramagnetic to hidden-order transition of URu2_2Si2_2

preprint2015arXivOpen access

Abstract

We report low-energy inelastic neutron scattering data of the paramagnetic (PM) to hidden-order (HO) phase transition at T0=17.5 KT_0=17.5\,{\rm K} in URu2_2Si2_2. While confirming previous results for the HO and PM phases, our data reveal a pronounced wavevector dependence of low-energy excitations across the phase transition. To analyze the energy scans we employ a damped harmonic oscillator model containing a fit parameter 1/Γ1/Γ which is expected to diverge at a second-order phase transition. Counter to expectations the excitations at Q⃗1=(1.44,0,0)\vec{Q}_1=(1.44,0,0) show an abrupt step-like suppression of 1/Γ1/Γ below T0T_0, whereas excitations at Q⃗0=(1,0,0)\vec{Q}_0=(1,0,0), associated with large-moment antiferromagnetism (LMAF) under pressure, show an enhancement and a pronounced peak of 1/Γ1/Γ at T0T_0. Therefore, at the critical HO temperature T0T_0, LMAF fluctuations become nearly critical as well. This is the behavior expected of a super-vector order parameter with nearly degenerate components for the HO and LMAF leading to nearly isotropic fluctuations in the combined order-parameter space.

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