Abstract

Quantum algorithms often assume independent spin qubits to produce trivial ∣↑⟩=∣0⟩|\uparrow\rangle=|0\rangle, ∣↓⟩=∣1⟩|\downarrow\rangle=|1\rangle mappings. This can be unrealistic in many solid-state implementations with sizeable magnetic interactions. Here we show that the lower part of the spectrum of a molecule containing three exchange-coupled metal ions with S=1/2S=1/2 and I=1/2I=1/2 is equivalent to nine electron-nuclear qubits. We derive the relation between spin states and qubit states in reasonable parameter ranges for the rare earth 159^{159}Tb3+^{3+} and for the transition metal Cu2+^{2+}, and study the possibility to implement Shor's Quantum Error Correction code on such a molecule. We also discuss recently developed molecular systems that could be adequate from an experimental point of view.

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