Possibility of valence-fluctuation mediated superconductivity in Cd-doped CeIrIn5_5 probed by In-NQR

preprint2012arXivOpen access

Abstract

We report on a pressure-induced evolution of exotic superconductivity and spin correlations in CeIr(In1−x_{1-x}Cdx_{x})5_5 by means of In-Nuclear-Quadrupole-Resonance (NQR) studies. Measurements of an NQR spectrum and nuclear-spin-lattice-relaxation rate 1/T11/T_1 have revealed that antiferromagnetism induced by the Cd-doping emerges locally around Cd dopants, but superconductivity is suddenly induced at TcT_c = 0.7 and 0.9 K at 2.34 and 2.75 GPa, respectively. The unique superconducting characteristics with a large fraction of the residual density of state at the Fermi level that increases with TcT_c differ from those for anisotropic superconductivity mediated by antiferromagnetic correlations. By incorporating the pressure dependence of the NQR frequency pointing to the valence change of Ce, we suggest that unconventional superconductivity in the CeIr(In1−x_{1-x}Cdx_{x})5_5 system may be mediated by valence fluctuations.

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