Persistent spin dynamics and absence of spin freezing in the HH-TT phase diagram of the 2D triangular antiferromagnet YbMgGaO4_4

preprint2020arXivOpen access

Abstract

We report results of muon spin relaxation and rotation (μμSR) experiments on the spin-liquid candidate~YbMgGaO4_{4}. No static magnetism ≳0.003μB\gtrsim 0.003μ_B per Yb ion, ordered or disordered, is observed down to 22~mK, a factor of two lower in temperature than previous measurements. Persistent (temperature-independent) spin dynamics are observed up to 0.20~K and at least 1~kOe, thus extending previous zero-field μμSR results over a substantial region of the HH-TT phase diagram. Knight shift measurements in a 10-kOe transverse field reveal two lines with nearly equal amplitudes. Inhomogeneous muon depolarization in a longitudinal field, previously characterized by stretched-exponential relaxation due to spatial inhomogeneity, is fit equally well with two exponentials, also of equal amplitudes. We attribute these results to two interstitial muon sites in the unit cell, rather than disorder or other spatial distribution. Further evidence for this attribution is found from agreement between the ratio of the two measured relaxation rates and calculated mean-square local Yb3+^{3+} dipolar fields at candidate muon sites. Zero-field data can be understood as a combination of two-exponential dynamic relaxation and quasistatic nuclear dipolar fields.

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