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Orbital Symmetry of Ba(Fe1-xCox)2As2 Superconductors Probed with X-ray Absorption Spectroscopy

The orbital symmetries of electron doped iron-arsenide superconductors Ba(Fe1-xCox)2As2 have been measured with x-ray absorption spectroscopy. The data reveal signatures of Fe d electron itinerancy, weak electronic correlations, and a high degree of Fe-As hybridization related to the bonding topology of the Fe dxz+yz states, which are found to contribute substantially at the Fermi level. The energies and detailed orbital character of Fe and As derived unoccupied s and d states are found to be in remarkably good agreement with the predictions of standard density functional theory.

preprint2010arXivOpen access
C. Parks CheneyF. BondinoT. A. CallcottP. VilmercatiD. EdererE. MagnanoM. MalvestutoF. ParmigianiA. S. SefatM. A. McGuireR. JinB. C. SalesD. MandrusD. J. SinghJ. W. FreelandN. Mannella
cond-mat.supr-concond-mat.str-el
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Open access16 authors2 topics
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C. Parks CheneyF. BondinoT. A. CallcottP. VilmercatiD. EdererE. MagnanoM. MalvestutoF. ParmigianiA. S. SefatM. A. McGuireR. JinB. C. SalesD. MandrusD. J. SinghJ. W. FreelandN. Mannella

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