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Optical read-out of the Néel vector in metallic antiferromagnet Mn$_{2}$Au

Metallic antiferromagnets with broken inversion symmetry on the two sublattices, strong spin-orbit coupling and high Néel temperatures offer new opportunities for applications in spintronics. Especially Mn$_{2}$Au, with high Néel temperature and conductivity, is particularly interesting for real-world applications. Here, manipulation of the orientation of the staggered magnetization,\textit{\ i.e.} the Néel vector, by current pulses has been recently demonstrated, with the read-out limited to studies of anisotropic magnetoresistance or X-ray magnetic linear dichroism. Here, we report on the in-plane reflectivity anisotropy of Mn$_{2}$Au (001) films, which were Néel vector aligned in pulsed magnetic fields. In the near-infrared, the anisotropy is $\approx$ 0.6\%, with higher reflectivity for the light polarized along the Néel vector. The observed magnetic linear dichroism is about four times larger than the anisotropic magnetoresistance. This suggests the dichroism in Mn$_{2}$Au is a result of the strong spin-orbit interactions giving rise to anisotropy of interband optical transitions, in-line with recent studies of electronic band-structure. The considerable magnetic linear dichroism in the near-infrared could be used for ultrafast optical read-out of the Néel vector in Mn$_{2}$Au.

preprint2021arXivOpen access

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