One-step approach to ARPES from strongly correlated solids: a Mott-Hubbard system

An expression is derived for angle-resolved photocurrent from a semi-infinite correlated system. Within the sudden approximation, the photocurrent is proportional to the spectral function of a one-particle two-time retarded Green's function $\mathcal{G}$ of an operator that creates an electron in a special quantum state $χ$ localized at the surface. For a system described by a many-body single-band model we present an analytical expression that relates the Green's function $\mathcal{G}$ with the Green's function of an infinite crystal $G_{b,\mathbf{k}}(ω)$ in Wannier representation. The role of final states and of the crystal surface is analysed for a model Green's function of the infinite crystal with a three-peak spectral function typical of a Mott-Hubbard metal. The momentum dependence of both the quasiparticle pole position and the spectral weight of the incoherent band manifest themselves in the shape of the photocurrent energy distribution curve.

No reviews yet.

No comments yet.