Abstract
The conventional understanding that a bandstructure that produces a Dirac delta function transport distribution (or transmission in the Landauer framework) maximizes the thermoelectric figure of merit, ZT, is revisited. Thermoelectric (TE) performance is evaluated using a simple tight binding (TB) model for electron dispersion and three different scattering models: 1) a constant scattering time, 2) a constant mean-free-path, and 3) a scattering rate proportional to the density-of-states. We found that a Dirac delta-function transmission never produces the maximum ZT. The best bandstructure for maximizing ZT depends on the scattering physics. These results demonstrate that the selection of bandstructure to maximize TE performance is more complex than previously thought and that a high density-of-states near the band edge does not necessarily improve TE performance.
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