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Observation of new intrinsic properties of VO2

The single crystal VO2, exihibiting a first-order metal-insulator transition (MIT) at 67.2 degrees C and an insulator-insulator transition (IIT) at ~49.7 degrees C, is grown. From synchrotron-based x-ray microdiffraction analysis, the IIT shows structural phase transition (SPT) of monoclinic M2 to M1 phases while the MIT displays M1 to rutile R phases. The IIT exhibits percolative SPT while the MIT shows abrupt transition width of < 0.02 degrees C, supporting Mott's prediction. The MIT occurs non-percolatively with a sharp boundary between R and M1 phases. The MIT onset temperature shows significant variation.

preprint2011arXivOpen access
Bongjin Simon MunKai ChenYoungchul LeemCatherine DejoieNobumichi TamuraMartin KunzZhi LiuMichael E. GrassChangwoo ParkY. Yvette LeeHonglyoul Ju
cond-mat.mtrl-sci
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Open access11 authors1 topic
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Bongjin Simon MunKai ChenYoungchul LeemCatherine DejoieNobumichi TamuraMartin KunzZhi LiuMichael E. GrassChangwoo ParkY. Yvette LeeHonglyoul Ju

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