Nuclear-order-induced quantum criticality and heavy-fermion superconductivity at ultra-low temperatures in YbRh2_2Si2_2

preprint2022arXivOpen access

Abstract

The tetragonal heavy-fermion metal YbRh2_2Si2_2 orders antiferromagnetically at TN=70T_{\rm N} = 70 mK and exhibits an unconventional quantum critical point (QCP) of Kondo-destroying type at BN=60B_{\rm N} = 60 mT, for the magnetic field applied within the basal (a,ba,b) plane. Ultra-low-temperature magnetization and heat-capacity measurements at very low fields indicate that the 4ff-electronic antiferromagnetic (AF) order is strongly suppressed by a nuclear-dominated hybrid order (`A-phase') at TA≤2.3T_{\rm A} \le 2.3 mK, such that quantum critical fluctuations develop at B≈0B \approx 0 (Schuberth et al., Science \textbf{351}, 485 (2016)). This enables the onset of heavy-fermion superconductivity (Tc=2T_{\rm c} = 2 mK) which appears to be suppressed by the primary AF order at elevated temperatures. Measurements of the Meissner effect reveal bulk superconductivity, with TcT_{\rm c} decreasing under applied field to Tc<1T_{\rm c} < 1 mK at B>20B > 20 mT. The observation of a weak but distinct superconducting shielding signal at a temperature as high as 10 mK suggests the formation of insulated random islands with emergent A-phase order and superconductivity. Upon cooling, the shielding signal increases almost linearly in temperature, indicating a growth of the islands which eventually percolate at T≈6.5T \approx 6.5 mK. Recent electrical-resistivity results by Nguyen et al. (Nat. Commun. \textbf{12}, 4341 (2021)) confirm the existence of superconductivity in YbRh2_2Si2_2 at ultra-low temperatures. The combination of the results of Schuberth et al. and Nguyen et al. at ultra-low temperatures below BNB_{\rm N}, along with those previously established at higher temperatures in the paramagnetic state, provide compelling evidence that the Kondo-destruction quantum criticality robustly drives unconventional superconductivity.

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