Nonequilibrium transport through magnetic vibrating molecules

preprint2013arXivOpen access

Abstract

We calculate the nonequilibrium conductance through a molecule or a quantum dot in which the occupation of the relevant electronic level is coupled with intensity λλ to a phonon mode, and also to two conducting leads. The system is described by the Anderson-Holstein Hamiltonian. We solve the problem using the Keldysh formalism and the non-crossing approximation (NCA) for both, the electron-electron and the electron-phonon interactions. We obtain a moderate decrease of the Kondo temperature TKT_K with λλ for fixed renormalized energy of the localized level Ed~\tilde{E_d}. The meaning and value of Ed~\tilde{E_d} are discussed. The spectral density of localized electrons shows in addition to the Kondo peak of width 2TK2 T_K, satellites of this peak shifted by multiples of the phonon frequency ω0 ω_0. The nonequilibrium conductance as a function of bias voltage VbV_b at small temperatures, also displays peaks at multiples of ω0ω_0 in addition to the central dominant Kondo peak near Vb=0V_b=0.

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