NMR relaxation in spin ice due to diffusing emergent monopoles

preprint2012arXivOpen access

Abstract

At low temperatures, spin dynamics in ideal spin ice is due mainly to dilute, thermally excited magnetic monopole excitations. I consider how these will affect the dynamics of a nuclear spin (the same theory applies to muon spin resonance if implanted muons do not diffuse). Up to the time scale for nearby monopoles to be rearranged, a stretched-exponential form of the relaxation functions is expected. I work out the expected exponent in that exponential and the formulas for the T1T_1 (longitudinal) and T2T_2 (dephasing) relaxations, as a function of the monopole density. Experimental NMR is incompatible with the predictions and I suggest is due to magnetic impurities.

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