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Nernst Effect as a Probe of Local Kondo Scattering in Heavy Fermions

A large, strongly temperature-dependent Nernst coefficient, $ν$, is observed between $T$ = 2 K and 300 K for CeCu$_2$Si$_2$ and Ce$_{0.8}$La$_{0.2}$Cu$_2$Si$_2$. The enhanced $ν(T)$ is determined by the asymmetry of the on-site Kondo (conduction electron$-4f$ electron) scattering rate. Taking into account the measured Hall mobility, $μ_H$, the highly unusual thermopower, $S$, of these systems can be semiquantitatively described by $S(T)$ $=$ $-$$ν(T)/μ_H(T)$, which explicitly demonstrates that the thermopower originates from the local Kondo scattering process over a wide temperature range from far above to well below the coherence temperature ($\approx$ 20 K for CeCu$_2$Si$_2$). Our results suggest that the Nernst effect can act as a proper probe of local charge-carrier scattering. This promises an impact on exploring the unconventional enhancement of the thermopower in correlated materials suited for potential applications.