Multiple lattice instabilities resolved by magnetic-field and disorder sensitivities in cubic paramagnetic phase of the orbital-degenerate frustrated spinel MgV2_2O4_4

preprint2014arXivOpen access

Abstract

Ultrasound velocity measurements of the orbital-degenerate frustrated spinel MgV2_2O4_4 are performed in the high-purity single crystal which exhibits successive structural and antiferromagnetic phase transitions, and in the disorder-introduced single crystal which exhibits spin-glass-like behavior. The measurements reveal that two-types of unusual temperature dependence of the elastic moduli coexist in the cubic paramagnetic phase, which are resolved by magnetic-field and disorder sensitivities: huge Curie-type softening with decreasing temperature, and concave temperature dependence with a characteristic minimum. These elastic anomalies suggest the coupling of lattice to coexisting orbital fluctuations and orbital-spin-coupled excitations.

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