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Metal enhanced fluorescence in rare earth doped plasmonic core-shell nanoparticles

We theoretically and numerically investigate metal enhanced fluorescence of plasmonic core-shell nanoparticles doped with rare earth (RE) ions. Particle shape and size are engineered to maximize the average enhancement factor (AEF) of the overall doped shell. We show that the highest enhancement (11 in the visible and 7 in the near-infrared) are achieved by tuning either the dipolar or quadrupolar particle resonance to the rare earth ions excitation wavelength. Additionally, the calculated AEFs are compared to experimental data reported in the literature, obtained in similar conditions (plasmon mediated enhancement) or when a metal-RE energy transfer mechanism is involved.

preprint2013arXivOpen access
S. DeromA. BerthelotA. PillonnetO. BenamaraA. M. JurdycC. GirardG. Colas des Francs
physics.atom-phcond-mat.mtrl-sciphysics.optics
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Open access7 authors3 topics
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S. DeromA. BerthelotA. PillonnetO. BenamaraA. M. JurdycC. GirardG. Colas des Francs

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