Many-body large polaron optical conductivity in SrTi1−x_{1-x}Nbx_xO3_3

preprint2010arXivOpen access

Abstract

Recent experimental data on the optical conductivity of niobium doped SrTiO3_{3} are interpreted in terms of a gas of large polarons with effective coupling constant αeff≈2α_{eff}\approx2. The {theoretical approach takes into account} many-body effects, the electron-phonon interaction with multiple LO-phonon branches, and the degeneracy and the anisotropy of the Ti t2g_{2g} conduction band. {Based on the Fröhlich interaction, the many-body large-polaron theory} provides an interpretation for the essential characteristics, except -- interestingly -- for the unexpectedly large intensity of a peak at ∼130\sim130 meV, of the observed optical conductivity spectra of SrTi1−x_{1-x}Nbx_{x}O3_{3} \textit{without} any adjustment of material parameters.

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