Magnetoelastic coupling and charge correlation lengths in a twin domain of Ba(Fe1−x_{1-x}Cox_{x})2_{2}As2_{2} (x=0.047x=0.047): A high-resolution X-ray diffraction study

preprint2013arXivOpen access

Abstract

The interplay between structure, magnetism and superconductivity in single crystal Ba(Fe1−x_{1-x}Cox_{x})2_{2}As2_{2} (x=0.047) has been studied using high-resolution X-ray diffraction by monitoring charge Bragg reflections in each twin domain separately. The emergence of the superconducting state is correlated with the suppression of the orthorhombic distortion around \emph{T}C_\texttt{C}, exhibiting competition between orthorhombicity and superconductivity. Above \emph{T}S_\texttt{S}, the in-plane charge correlation length increases with the decrease of temperature, possibly induced by nematic fluctuations in the paramagnetic tetragonal phase. Upon cooling, anomalies in the in-plane charge correlation lengths along aa (ξaξ_{a}) and bb axes (ξbξ_{b}) are observed at \emph{T}S_\texttt{S} and also at \emph{T}N_\texttt{N} indicative of strong magnetoelastic coupling. The in-plane charge correlation lengths are found to exhibit anisotropic behavior along and perpendicular to the in-plane component of stripe-type AFM wave vector (101)O_{\rm O} below around \emph{T}N_\texttt{N}. The temperature dependence of the out-of-plane charge correlation length shows a single anomaly at \emph{T}N_\texttt{N}, reflecting the connection between Fe-As distance and Fe local moment. The origin of the anisotropic in-plane charge correlation lengths ξaξ_{a} and ξbξ_{b} is discussed on the basis of the antiphase magnetic domains and their dynamic fluctuations.

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