Abstract

We report results of a magneto-optical investigation of the Zintl-phase compound EuIn2_2P2_2. The compound orders magnetically at TCT_C=24 K and exhibits concomitant large magnetoresistance effects. For T≤T\le50 K and increasing magnetic fields we observe a transfer of spectral weight in σ1(ω)σ_1(ω) from energies above 1 eV into the low-energy metallic component as well as into a mid-infrared signal centered at about 600 cm−1^{-1}. This latter absorption is reminiscent to what has been seen in a large variety of so-called Kondo materials and ascribed to excitations across the hybridization gap. The observed gain of Drude weight upon increasing magnetic field suggests an enhancement of the itinerant charge-carrier concentration due to the increasing magnetization, a phenomenon that was previously observed in other compounds which exhibit colossal magnetoresistive effects.

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