Magnetization reversal, giant exchange bias effect and magnetoresistance in oxygen vacancy ordered Sr4_{4}Fe3_{3}CoO11_{11}

preprint2019arXivOpen access

Abstract

We report the structural, magnetic, exchange bias and magnetotransport effect in Sr4_{4}Fe3_{3}CoO11_{11}. The material crystallizes in the orthorhombic Cmmm\textit{Cmmm} space group. It shows antiferromagnetic (G-type) transition (TN_{N} = 255 K) along with interesting temperature induced magnetization reversal (TComp._{Comp.}= 47 K measured at 100 Oe). The magnetic reversal can be elucidated considering the increased magnetocrystalline anisotropy with Co substitution. Magnetoresistance measurements shows an interesting crossover from negative to positive side at ∼\sim 100 K. The negative magnetoresistance reaches 80 %\% at 25 K in 7 T magnetic field. Giant exchange bias effect is observed below TN_{N} under field cooling condition. The origin of the negative magnetoresistance and giant exchange bias in this sample can be attributed to the magnetic frustration.

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