Magnetization process and ordering of the S=1/2S=1/2 pyrochlore magnet in a field

preprint2022arXivOpen access

Abstract

We study the S=1/2S=1/2 pyrochlore Heisenberg antiferromagnet in a magnetic field. Using large scale density-matrix renormalization group (DMRG) calculations for clusters up to 128128 spins, we find indications for a finite triplet gap, causing a threshold field to nonzero magnetization in the magnetization curve. We obtain a robust saturation field consistent with a magnon crystal, although the corresponding 5/65/6 magnetization plateau is very slim and possibly unstable. Most remarkably, there is a pronounced and apparently robust 12\frac 1 2 magnetization plateau where the groundstate breaks (real-space) rotational symmetry, exhibiting oppositely polarised spins on alternating kagome and triangular planes. Reminiscent of the kagome ice plateau of the pyrochlore Ising magnet known as spin ice, it arises via a much more subtle `quantum order by disorder' mechanism.

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